Sediment from urban impervious surfaces has the potential to be an important vector for contaminants, particularly where stormwater culverts and other buried channels draining large impervious areas exit from underground pipes into open channels. To better understand urban sediment sources and their relation to fallout radionuclides, we collected samples of rainfall, urban sediment (pavement sediment, topsoil), streambank sediment, and fluvial sediment (suspended sediment and bed sediment) for ⁷Be, ²¹⁰Pb_ex, and ¹³⁷Cs analysis. The results indicate that each rainfall event tags pavement sediment with elevated activities of ⁷Be and ²¹⁰Pb_ex such that runoff from impervious surfaces in the buried channel part of the stream network contains the highest activities. Pavement sediment, because it is characteristically a thin veneer, has a small mass to rainwater ratio resulting in a greater tagging of ⁷Be and ²¹⁰Pb_ex activity than does topsoil on a per gram basis. An unmixing model indicated that suspended-sediment samples collected at the culvert outlet from the buried-channel network are from pavement sediment sources (45 ± 25%) with a smaller component of topsoil (22 ± 19%), and a component from streambanks (32 ± 35%) that we infer to be older channel material and subsoil eroded from within the culvert system. Downstream from the culvert, suspended sediment collected from the open-channel parts of the stream had ⁷Be and ²¹⁰Pb_ex activities that were substantially reduced by the contribution of sediment from streambanks (57 ± 15%), with pavement contributions decreasing to 15 (±9%) and topsoil contributing 28 (±7%). The results highlight the utility of ⁷Be, ²¹⁰Pb_ex, and ¹³⁷Cs as tracers of urban sediment sources, resulting in a unique radionuclide signature for urban watersheds compared to other sediment-source settings.